Regarding the CO analyzer, they're certified to be accurate to a very small deviation, much, much more accurate than what we even need. As a matter of fact, even though I haven't used mine, yet, I already received a notice from the seller stating my meter is due for recertification. I'm not concerned with it. If I "top out" the analyzer, I'm positive I'll be good to go, even if it is off a small amount.
You have N available to you? I'd go with that. CO is very deadly. Each year many people succumb to it in their homes while sleeping due to faulty furnaces and plugged up chimneys, and I'm certain that the amounts they die from are far, far less than the amounts that (we) can purposely generate from burning charcoal and collecting the produced CO in a small space. The one thing those people have going for them is that they are asleep, so they don't even realize death is coming. It would be difficult to replicate that intentionally, though. The closest and easiest way is to get the CO level really high, so that we can replicate that "sleeping" state by rendering ourselves unconscious quickly, so that we have no idea of when death comes.
I think poisons were popular back in the day. And they were probably very painful deaths, too. I guess there were fewer suicides ages ago, at least by a total number count, but I'm not sure if the numbers would be that much less, if less at all, if you could calculate them on a per capita basis.