It's not a reliable way. I took 20-30 Xanax 2mg tabs and I just woke up in hospital. I don't think they even had to really do anything to me as it's just so safe in overdose.
I think that in order for it to be lethal, you would have to mix a lot of it with alcohol, as the LD50 would require you to take several thousands times the normal dosage. I wouldn't recommend that either personally, as looking at the side effects it seems to be a pretty painful OD. I wouldn't want you to be in any pain so I would consider something else if at all possible.
A benzo overdose is rarely fatal in itself. Knocking a lot back with vodka may work. Adding a third sedative like z-drugs or opiates would increase the likelihood of success further.
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